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Two methods for mitigating unacceptably high HCCI heat-release rates are investigated and compared in this combined experimental/CFD work. Retarding the combustion phasing by decreasing the intake temperature is found to have good potential for smoothing heat-release rates and reducing engine knock. There are at least three reasons for this: 1) lower combustion temperatures, 2) less pressure rise when the combustion is occurring during the expansion stroke, and 3) the natural thermal stratification increases around TDC. However, overly retarded combustion leads to unstable operation with partial-burn cycles resulting in high IMEPg variations and increased emissions. Enhanced natural thermal stratification by increased heat-transfer rates was explored by lowering the coolant temperature from 100 to 50°C. This strategy substantially decreased the heat-release rates and lowered the knocking intensity under certain conditions.

The development of detailed chemical kinetic reaction mechanisms for analysis of autoignition and knocking of complex hydrocarbon fuels is described. The wide ranges of temperature and pressure which are encountered by end gases in automobile engine combustion chambers result in extreme demands on the reaction mechanisms intended to describe knocking conditions. The reactions and chemical species which are most important in each temperature and pressure regime are discussed, and the validation of these reaction mechanisms through comparison with idealized experimental results is described. The use of these mechanisms is illustrated through comparisons between computed results and experimental data obtained in actual knocking engines.

The development of detailed chemical kinetic reaction mechanisms for analysis of autoignition and knocking of hydrocarbon fuels is described. In particular, kinetic processes of concern for the oxidation of complex hydrocarbon fuel molecules are emphasized. The wide ranges of temperature and pressure which are encountered by end gases in automobile engine combustion chambers result in extreme demands on reaction mechanisms which are intended to describe knocking conditions and predict rates of combustion and ignition. The reactions and chemical species which are most important in each temperature and pressure regime are discussed, and the validation of these reaction mechanisms through comparison with idealized experimental results is described.

Homogeneous Charge Compression Ignition (HCCI) combustion is a process dominated by chemical kinetics of the fuel-air mixture. The hottest part of the mixture ignites first, and compresses the rest of the charge, which then ignites after a short time lag. Crevices and boundary layers generally remain too cold to react, and result in substantial hydrocarbon and carbon monoxide emissions. Turbulence has little effect on HCCI combustion, and may be most important as a factor in determining temperature gradients and boundary layer thickness inside the cylinder. The importance of thermal gradients inside the cylinder makes it necessary to use an integrated fluid mechanics-chemical kinetics code for accurate predictions of HCCI combustion. However, the use of a fluid mechanics code with detailed chemical kinetics is too computationally intensive for today's computers.

Laminar burning velocity (LBV) measurements are reported for promising high-performance fuels selected as drop-in transportation fuels to automotive grade gasoline as part of the United States Department of Energy’s Co-Optimization of Fuels and Engines Initiative (Co-Optima). LBV measurements were conducted for ethanol, methyl acetate, and 2-methylfuran with synthetic air (79.0 % N2 and 21.0 % O2 by volume) within a constant-volume spherical combustion rig. Mixture initial temperature was fixed at 428±4 K, with the corresponding initial pressure of 1.00±0.02 atm. Current LBV of ethanol is in good agreement with literature data. LBV of ethanol and 2-methylfuran showed similar values over the range of equivalence ratios, while methyl acetate exhibited an LBV significantly lower over the range of tested equivalence ratios. The maximum laminar burning velocity occurred at slightly richer equivalence ratio from the stoichiometric value for all fuels tested.

A phenomenological description, or “conceptual model,” of how direct-injection (DI) diesel combustion occurs has been derived from laser-sheet imaging and other recent optical data. To provide background, the most relevant of the recent imaging data of the author and co-workers are presented and discussed, as are the relationships between the various imaging measurements. Where appropriate, other supporting data from the literature is also discussed. Then, this combined information is summarized in a series of idealized schematics that depict the combustion process for a typical, modern-diesel-engine condition. The schematics incorporate virtually all of the information provided by our recent imaging data including: liquid- and vapor-fuel zones, fuel/air mixing, autoignition, reaction zones, and soot distributions.

The homogeneous charge, compression-ignition (HCCI) combustion process has the potential to significantly reduce NOx and particulate emissions, while achieving high thermal efficiency and the capability of operating with a wide variety of fuels. This makes the HCCI engine an attractive technology that can ostensibly provide diesel-like fuel efficiency and very low emissions, which may allow emissions compliance to occur without relying on lean aftertreatment systems.